No, in fact they're both quite good for you in many ways.
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The best way to take it is to take a !:1 calcium citrate to magnesium citrate. Solaray makes one. The normal ration is 2:1 calcium to magnesium. Taking it this way ensures you don't upset the balance between calcium and magnesium when you up your magnesium levels. As to whether it alone will cure your anxiety, probably not, bit it is an essential nutrient for relaxation. Fish oil is more associated with helping depression than anxiety, but most anxious people get depressed and most depressed people get anxious, so it couldn't hurt. For an idea of what a total supplementation program might look like, read Natural Highs by Hyla Cass, a psychiatrist at UCLA.